标題: Enhanced dewaterability of sewage sludge by Fe2+-activated persulfate oxidation under mild temperature
作者: Xiong, Q (Xiong, Qiao); Zhou, M (Zhou, Min); Liu, MJ (Liu, Mengjia); Han, Y (Han, Yi); Hou, HB (Hou, Haobo)
來源出版物:DESALINATION AND WATER TREATMENT卷:94頁碼:100-108 DOI:10.5004/dwt.2017.21482 出版年: OCT 2017
摘要:We investigated the improvement in dewaterability of sewage sludge by two-valent iron activated persulfate oxidation process under mild temperature. Sludge dewaterability was found to be improved in this system. Capillary suction time (CST) and setting property were used to characterize sludge dewatering. Zeta potential, Fourier-transformed infrared (FT-IR) spectroscopy, scanning electronic microscopy (SEM), three-dimensional excitation-emission matrix (EEM) fluorescence spectroscopy, thermogravimetry (TG) and differential scanning calorimetry (DSC) analyses were used to explore influencing mechanisms. The optimal conditions to achieve the highest CST reduction efficiency (95.3% reduction within 3 min) in room temperature were found to be 62.9 mg persulfate (S2O82-) g(-1) dry solid (DS), 19.6 mg Fe2+ g(-1) DS, and pH 5. SEM images revealed the rupture of sludge flocs; EEM, TG-DSC, and FT-IR analyses indicated that the degradation of protein-like and polysaccharide-like substances in extracellular polymeric substances (EPS), which contributed to the release of EPS-bound water and interstitial water trapped between flocs, as well as subsequent enhanced dewaterability.
入藏号:WOS:000418866700011
文獻類型:Article
語種:English
作者關鍵詞:Sewage sludge; Dewaterability; Two-valent iron; Persulfate oxidation
擴展關鍵詞: EXTRACELLULAR POLYMERIC SUBSTANCES; WASTE ACTIVATED-SLUDGE; ZERO-VALENT IRON; HYDROXYL RADICALS; WATER SLUDGE; DEGRADATION; PRETREATMENT; KINETICS; SULFATE; METALS
通訊作者地址:Hou, HB (reprint author), Wuhan Univ, Sch Resource & Environm Sci, Wuhan 430072, Hubei, Peoples R China.
Hou, HB (reprint author), Hubei Environm Remediat Mat Engn Technol Res Ctr, Wuhan 430072, Hubei, Peoples R China.
電子郵件地址: whuxiongqiao@163.com; zhoumin@whu.edu.cn; whuliumengjia@163.com; yihan@whu.edu.cn; hhb-bhh@163.com
地址:
[Xiong, Qiao; Zhou, Min; Liu, Mengjia; Han, Yi; Hou, Haobo] Wuhan Univ, Sch Resource & Environm Sci, Wuhan 430072, Hubei, Peoples R China.
[Xiong, Qiao; Hou, Haobo] Hubei Environm Remediat Mat Engn Technol Res Ctr, Wuhan 430072, Hubei, Peoples R China.
影響因子:1.631
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